Unconventional spin density wave in (TMTSF)2PF6 below T* ~ 4K

The presence of subphases in spin-density wave (SDW) phase of (TMTSF)2PF6 below T* ~ 4K has been suggested by several experiments but the nature of the new phase is still controversial. We have investigated the temperature dependence of the angular dependence of the magnetoresistance in the SDW phase which shows different features for temperatures above and below T*. For T > 4K the magnetoresistance can be understood in terms of the Landau quantization of the quasiparticle spectrum in a magnetic field, where the imperfect nesting plays the crucial role. We propose that below T* ~ 4K the new unconventional SDW (USDW) appears modifying dramatically the quasiparticle spectrum. Unlike conventional SDW the order parameter of USDW depends on the quasiparticle momentum. The present model describes many features of the angular dependence of magnetoresistance reasonably well. Therefore, we may conclude that the subphase in (TMTSF)2PF6 below T* ~ 4K is described as SDW plus USDW.Comment: 7 pages, 9 figures, RevTeX4; misprint corrected, references updated, a few sentences adde

Anisotropic Charge Modulation in Ladder Planes of Sr_14-xCa_xCu_24O_41

The charge response of the ladders in Sr_14-xCa_xCu_24O_41 is characterized by dc resistivity, low frequency dielectric and optical spectroscopy in all three crystallographic directions. The collective charge-density wave screened mode is observed in the direction of the rungs for x=0, 3 and 6, in addition to the mode along the legs. For x=8 and 9, the charge-density-wave response along the rungs fully vanishes, while the one along the legs persists. The transport perpendicular to the planes is always dominated by hopping.Comment: 4 pages, 3 figures, submitted to PRB R

The angular dependent magnetoresistance in alpha-(BEDT-TTF)_2KHg(SCN)_4

In spite of extensive experimental studies of the angular dependent magnetoresistance (ADMR) of the low temperature phase (LTP) of alpha-(BEDT-TTF)_2KHg(SCN)_4 about a decade ago, the nature of LTP remains elusive. Here we present a new study of ADMR of LTP in alpha-(ET)_2 salts assuming that LTP is unconventional charge density wave (UCDW). In the presence of magnetic field the quasiparticle spectrum in UCDW is quantized, which gives rise to striking ADMR in UCDW. The present model appears to account for many existing ADMR data of alpha-(BEDT-TTF)_2KHg(SCN)_4 remarkably well.Comment: 6 pages, 4 figure

Klizni valovi spinske gustoce: proučavanje strujnog šuma, ovisnosti o magnetskom polju i Hallovog otpora

We have studied the current-voltage characteristics of the (TMTSF)2PF6 in the spin density state (SDW), and in zero and finite external magnetic field. For the oscillating part of the nonlinear voltage response to the applied DC electric field, the fundamental frequency distribution (as a function of this field) and a nonlinear relation between the frequency and the SDW current reveal the growth of parallel conduction channels characterized by lower velocities and larger cross-sections. The number of fundamental frequencies, their amplitude and the level of low-frequency noise as well as the depinning behaviour provide a consistent indication of the sample inhomogeneities and associated local field variations, and might be well understood within the framework of the phase slippage model. The increase of the threshold electric field with the applied magnetic filed can be explained by the Bjeli-Maki theory, if the imperfect nesting is taken into account. Finally, the electric-field dependence of the Hall resistivity is consistent with the sliding mechanism of the SDW conduction.Proučavali smo karakteristike napon – struja materijala (TMTSF)2PF6 u stanju valova spinske gustoće (SDW). Za oscilatorni dio nelinearnog naponskog odziva na istosmjerno električno polje, osnovna frekventna raspodjela (kao funkcija tog polja) i nelinearan odnos frekvencije i SDW struje pokazuju rast usporednih kanala vođenja označenih manjim brzinama i većim udarnim presjecima. Broj osnovnih frekvencija, njihove amplitude i razina niskofrekventnog šuma, kao i otkočno ponašanje sustavno pokazuju na nehomogenosti uzorka i pridružene varijacije lokalnog polja, i mogu se shvatiti u okviru modela klizne faze. Rast praga električnog polja s magnetskim poljem može se protumačiti Bjeliš-Makijevom teorijom, ako se uzme u obzir ugniježdenje. Konačno, nalazimo da je ovisnost Hallovog otpora o električnom polju u skladu s kliznim mehanizmom SDW vođenja struje

Klizni valovi spinske gustoce: proučavanje strujnog šuma, ovisnosti o magnetskom polju i Hallovog otpora

We have studied the current-voltage characteristics of the (TMTSF)2PF6 in the spin density state (SDW), and in zero and finite external magnetic field. For the oscillating part of the nonlinear voltage response to the applied DC electric field, the fundamental frequency distribution (as a function of this field) and a nonlinear relation between the frequency and the SDW current reveal the growth of parallel conduction channels characterized by lower velocities and larger cross-sections. The number of fundamental frequencies, their amplitude and the level of low-frequency noise as well as the depinning behaviour provide a consistent indication of the sample inhomogeneities and associated local field variations, and might be well understood within the framework of the phase slippage model. The increase of the threshold electric field with the applied magnetic filed can be explained by the Bjeli-Maki theory, if the imperfect nesting is taken into account. Finally, the electric-field dependence of the Hall resistivity is consistent with the sliding mechanism of the SDW conduction.Proučavali smo karakteristike napon – struja materijala (TMTSF)2PF6 u stanju valova spinske gustoće (SDW). Za oscilatorni dio nelinearnog naponskog odziva na istosmjerno električno polje, osnovna frekventna raspodjela (kao funkcija tog polja) i nelinearan odnos frekvencije i SDW struje pokazuju rast usporednih kanala vođenja označenih manjim brzinama i većim udarnim presjecima. Broj osnovnih frekvencija, njihove amplitude i razina niskofrekventnog šuma, kao i otkočno ponašanje sustavno pokazuju na nehomogenosti uzorka i pridružene varijacije lokalnog polja, i mogu se shvatiti u okviru modela klizne faze. Rast praga električnog polja s magnetskim poljem može se protumačiti Bjeliš-Makijevom teorijom, ako se uzme u obzir ugniježdenje. Konačno, nalazimo da je ovisnost Hallovog otpora o električnom polju u skladu s kliznim mehanizmom SDW vođenja struje

Unconventional charge density wave in the organic conductor alpha-(BEDT-TTF)_2KHg(SCN)_4

The low temperature phase (LTP) of alpha-(BEDT-TTF)_2KHg(SCN)_4 salt is known for its surprising angular dependent magnetoresistance (ADMR), which has been studied intensively in the last decade. However, the nature of the LTP has not been understood until now. Here we analyse theoretically ADMR in unconventional (or nodal) charge density wave (UCDW). In magnetic field the quasiparticle spectrum in UCDW is quantized, which gives rise to spectacular ADMR. The present model accounts for many striking features of ADMR data in alpha-(BEDT-TTF)_2KHg(SCN)_4.Comment: 5 pages, 6 figure

Anisotropic charge dynamics in the quantum spin-liquid candidate κ\kappa-(BEDT-TTF)2_2Cu2_2(CN)3_3

We have in detail characterized the anisotropic charge response of the dimer Mott insulator $\kappa$-(BEDT-TTF)$_2$\-Cu$_2$(CN)$_3$ by dc conductivity, Hall effect and dielectric spectroscopy. At room temperature the Hall coefficient is positive and close to the value expected from stoichiometry; the temperature behavior follows the dc resistivity $\rho(T)$. Within the planes the dc conductivity is well described by variable-range hopping in two dimensions; this model, however, fails for the out-of-plane direction. An unusually broad in-plane dielectric relaxation is detected below about 60 K; it slows down much faster than the dc conductivity following an Arrhenius law. At around 17 K we can identify a pronounced dielectric anomaly concomitantly with anomalous features in the mean relaxation time and spectral broadening. The out-of-plane relaxation, on the other hand, shows a much weaker dielectric anomaly; it closely follows the temperature behavior of the respective dc resistivity. At lower temperatures, the dielectric constant becomes smaller both within and perpendicular to the planes; also the relaxation levels off. The observed behavior bears features of relaxor-like ferroelectricity. Because heterogeneities impede its long-range development, only a weak tunneling-like dynamics persists at low temperatures. We suggest that the random potential and domain structure gradually emerge due to the coupling to the anion network.Comment: 14 pages, 13 figure